As a noun, complement means "anything that completes or perfects." As a verb, complement means "to make complete" or "to enhance."

A complement of four students would bring our class up to its normal size, [noun] That teal blouse complements your jacket nicely, [verb]

As a noun, compliment means "something said in admiration, praise, or flattery." As a verb, compliment means "to congratulate" or "to praise."

Jeff's mother complimented him on the job he had done cleaning his room, [verb] The compliment from his mother boosted Jeff's morale, [noun]

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